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fix_langevin_drude.cpp
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Mon, Nov 11, 03:53

fix_langevin_drude.cpp

/* ----------------------------------------------------------------------
LAMMPS - Large-scale Atomic/Molecular Massively Parallel Simulator
http://lammps.sandia.gov, Sandia National Laboratories
Steve Plimpton, sjplimp@sandia.gov
Copyright (2003) Sandia Corporation. Under the terms of Contract
DE-AC04-94AL85000 with Sandia Corporation, the U.S. Government retains
certain rights in this software. This software is distributed under
the GNU General Public License.
See the README file in the top-level LAMMPS directory.
------------------------------------------------------------------------- */
#include <string.h>
#include <stdlib.h>
#include <math.h>
#include "fix_langevin_drude.h"
#include "atom.h"
#include "force.h"
#include "comm.h"
#include "input.h"
#include "variable.h"
#include "random_mars.h"
#include "group.h"
#include "update.h"
#include "modify.h"
#include "compute.h"
#include "error.h"
#include "domain.h"
using namespace LAMMPS_NS;
using namespace FixConst;
enum{NOBIAS,BIAS};
enum{CONSTANT,EQUAL};
/* ---------------------------------------------------------------------- */
FixLangevinDrude::FixLangevinDrude(LAMMPS *lmp, int narg, char **arg) :
Fix(lmp, narg, arg)
{
if (narg < 9) error->all(FLERR,"Illegal fix langevin/drude command");
// TODO add option for tally
// Langevin thermostat should be applied every step
nevery = 1;
global_freq = nevery;
comm_reverse = 3;
// core temperature
tstr_core = NULL;
if (strstr(arg[3],"v_") == arg[3]) {
int n = strlen(&arg[3][2]) + 1;
tstr_core = new char[n];
strcpy(tstr_core,&arg[3][2]);
tstyle_core = EQUAL;
} else {
t_start_core = force->numeric(FLERR,arg[3]);
t_target_core = t_start_core;
tstyle_core = CONSTANT;
}
t_period_core = force->numeric(FLERR,arg[4]);
int seed_core = force->inumeric(FLERR,arg[5]);
// drude temperature
tstr_drude = NULL;
if (strstr(arg[7],"v_") == arg[6]) {
int n = strlen(&arg[6][2]) + 1;
tstr_drude = new char[n];
strcpy(tstr_drude,&arg[6][2]);
tstyle_drude = EQUAL;
} else {
t_start_drude = force->numeric(FLERR,arg[6]);
t_target_drude = t_start_drude;
tstyle_drude = CONSTANT;
}
t_period_drude = force->numeric(FLERR,arg[7]);
int seed_drude = force->inumeric(FLERR,arg[8]);
// error checks
if (t_period_core <= 0.0)
error->all(FLERR,"Fix langevin/drude period must be > 0.0");
if (seed_core <= 0) error->all(FLERR,"Illegal langevin/drude seed");
if (t_period_drude <= 0.0)
error->all(FLERR,"Fix langevin/drude period must be > 0.0");
if (seed_drude <= 0) error->all(FLERR,"Illegal langevin/drude seed");
random_core = new RanMars(lmp,seed_core);
random_drude = new RanMars(lmp,seed_drude);
int iarg = 9;
zero = 0;
while (iarg < narg) {
if (strcmp(arg[iarg],"zero") == 0) {
if (iarg+2 > narg) error->all(FLERR,"Illegal fix langevin/drude command");
if (strcmp(arg[iarg+1],"no") == 0) zero = 0;
else if (strcmp(arg[iarg+1],"yes") == 0) zero = 1;
else error->all(FLERR,"Illegal fix langevin/drude command");
iarg += 2;
} else error->all(FLERR,"Illegal fix langevin/drude command");
}
tflag = 0; // no external compute/temp is specified yet (for bias)
energy = 0.;
fix_drude = NULL;
temperature = NULL;
id_temp = NULL;
}
/* ---------------------------------------------------------------------- */
FixLangevinDrude::~FixLangevinDrude()
{
delete random_core;
delete [] tstr_core;
delete random_drude;
delete [] tstr_drude;
}
/* ---------------------------------------------------------------------- */
int FixLangevinDrude::setmask()
{
int mask = 0;
mask |= POST_FORCE;
return mask;
}
/* ---------------------------------------------------------------------- */
void FixLangevinDrude::init()
{
// check variable-style target core temperature
if (tstr_core) {
tvar_core = input->variable->find(tstr_core);
if (tvar_core < 0)
error->all(FLERR,"Variable name for fix langevin/drude does not exist");
if (input->variable->equalstyle(tvar_core)) tstyle_core = EQUAL;
else error->all(FLERR,"Variable for fix langevin/drude is invalid style");
}
// check variable-style target drude temperature
if (tstr_drude) {
tvar_drude = input->variable->find(tstr_drude);
if (tvar_drude < 0)
error->all(FLERR,"Variable name for fix langevin/drude does not exist");
if (input->variable->equalstyle(tvar_drude)) tstyle_drude = EQUAL;
else error->all(FLERR,"Variable for fix langevin/drude is invalid style");
}
int ifix;
for (ifix = 0; ifix < modify->nfix; ifix++)
if (strcmp(modify->fix[ifix]->style,"drude") == 0) break;
if (ifix == modify->nfix) error->all(FLERR, "fix langevin/drude requires fix drude");
fix_drude = (FixDrude *) modify->fix[ifix];
}
/* ---------------------------------------------------------------------- */
void FixLangevinDrude::setup(int vflag)
{
if (!strstr(update->integrate_style,"verlet"))
error->all(FLERR,"RESPA style not compatible with fix langevin/drude");
if (!comm->ghost_velocity)
error->all(FLERR,"fix langevin/drude requires ghost velocities. Use comm_modify vel yes");
if (zero) {
int *mask = atom->mask;
int nlocal = atom->nlocal;
int *drudetype = fix_drude->drudetype;
int *type = atom->type;
bigint ncore_loc = 0;
for (int i=0; i<nlocal; i++)
if (mask[i] & groupbit && drudetype[type[i]] != DRUDE_TYPE)
ncore_loc++;
MPI_Allreduce(&ncore_loc, &ncore, 1, MPI_LMP_BIGINT, MPI_SUM, world);
}
}
/* ---------------------------------------------------------------------- */
int FixLangevinDrude::modify_param(int narg, char **arg)
{
if (strcmp(arg[0],"temp") == 0) {
if (narg < 2) error->all(FLERR,"Illegal fix_modify command");
delete [] id_temp;
int n = strlen(arg[1]) + 1;
id_temp = new char[n];
strcpy(id_temp,arg[1]);
int icompute = modify->find_compute(id_temp);
if (icompute < 0)
error->all(FLERR,"Could not find fix_modify temperature ID");
temperature = modify->compute[icompute];
if (temperature->tempflag == 0)
error->all(FLERR,
"Fix_modify temperature ID does not compute temperature");
if (temperature->igroup != igroup && comm->me == 0)
error->warning(FLERR,"Group for fix_modify temp != fix group");
return 2;
}
return 0;
}
/* ---------------------------------------------------------------------- */
void FixLangevinDrude::post_force(int /*vflag*/)
{
// Thermalize by adding the langevin force if thermalize=true.
// Each core-Drude pair is thermalized only once: where the core is local.
double **v = atom->v, **f = atom->f;
int *mask = atom->mask;
int nlocal = atom->nlocal, nall = atom->nlocal + atom->nghost;
int *type = atom->type;
double *mass = atom->mass;
double *rmass = atom->rmass;
double ftm2v = force->ftm2v, mvv2e = force->mvv2e;
double kb = force->boltz, dt = update->dt;
int *drudetype = fix_drude->drudetype;
tagint *drudeid = fix_drude->drudeid;
double vdrude[3], vcore[3]; // velocities in reduced representation
double fdrude[3], fcore[3]; // forces in reduced representation
double Ccore, Cdrude, Gcore, Gdrude;
double fcoresum[3], fcoreloc[3];
int dim = domain->dimension;
// Compute target core temperature
if (tstyle_core == CONSTANT)
t_target_core = t_start_core; // + delta * (t_stop-t_start_core);
else {
modify->clearstep_compute();
t_target_core = input->variable->compute_equal(tvar_core);
if (t_target_core < 0.0)
error->one(FLERR, "Fix langevin/drude variable returned "
"negative core temperature");
modify->addstep_compute(update->ntimestep + nevery);
}
// Compute target drude temperature
if (tstyle_drude == CONSTANT)
t_target_drude = t_start_drude; // + delta * (t_stop-t_start_core);
else {
modify->clearstep_compute();
t_target_drude = input->variable->compute_equal(tvar_drude);
if (t_target_drude < 0.0)
error->one(FLERR, "Fix langevin/drude variable returned "
"negative drude temperature");
modify->addstep_compute(update->ntimestep + nevery);
}
// Clear ghost forces
// They have already been communicated if needed
for (int i = nlocal; i < nall; i++) {
for (int k = 0; k < dim; k++)
f[i][k] = 0.;
}
if (zero) for (int k=0; k<dim; k++) fcoreloc[k] = 0.;
// NB : the masses are the real masses, not the reduced ones
for (int i = 0; i < nlocal; i++) {
if (mask[i] & groupbit) { // only the cores need to be in the group
if (drudetype[type[i]] == NOPOL_TYPE) { // Non-polarizable atom
double mi;
if (rmass)
mi = rmass[i];
else
mi = mass[type[i]];
Gcore = mi / t_period_core / ftm2v;
Ccore = sqrt(2.0 * Gcore * kb * t_target_core / dt / ftm2v / mvv2e);
if (temperature) temperature->remove_bias(i, v[i]);
for(int k = 0; k < dim; k++){
fcore[k] = Ccore * random_core->gaussian() - Gcore * v[i][k];
if (zero) fcoreloc[k] += fcore[k];
f[i][k] += fcore[k];
}
if (temperature) temperature->restore_bias(i, v[i]);
} else {
if (drudetype[type[i]] == DRUDE_TYPE) continue; // do with the core
int j = atom->map(drudeid[i]);
double mi, mj, mtot, mu; // i is core, j is drude
if (rmass) {
mi = rmass[i];
mj = rmass[j];
} else {
mi = mass[type[i]];
mj = mass[type[j]];
}
mtot = mi + mj;
mu = mi * mj / mtot;
mi /= mtot;
mj /= mtot;
Gcore = mtot / t_period_core / ftm2v;
Gdrude = mu / t_period_drude / ftm2v;
Ccore = sqrt(2.0 * Gcore * kb * t_target_core / dt / ftm2v / mvv2e);
Cdrude = sqrt(2.0 * Gdrude * kb * t_target_drude / dt / ftm2v / mvv2e);
if (temperature) {
temperature->remove_bias(i, v[i]);
temperature->remove_bias(j, v[j]);
}
for (int k=0; k<dim; k++) {
// TODO check whether a fix_modify temp can subtract a bias velocity
vcore[k] = mi * v[i][k] + mj * v[j][k];
vdrude[k] = v[j][k] - v[i][k];
fcore[k] = Ccore * random_core->gaussian() - Gcore * vcore[k];
fdrude[k] = Cdrude * random_drude->gaussian() - Gdrude * vdrude[k];
if (zero) fcoreloc[k] += fcore[k];
f[i][k] += mi * fcore[k] - fdrude[k];
f[j][k] += mj * fcore[k] + fdrude[k];
// TODO tally energy if asked
}
if (temperature) {
temperature->restore_bias(i, v[i]);
temperature->restore_bias(j, v[j]);
}
}
}
}
if(zero) { // Remove the drift
MPI_Allreduce(fcoreloc, fcoresum, dim, MPI_DOUBLE, MPI_SUM, world);
for (int k=0; k<dim; k++) fcoresum[k] /= ncore;
for (int i=0; i<nlocal; i++) {
if (mask[i] & groupbit) { // only the cores need to be in the group
if (drudetype[type[i]] == NOPOL_TYPE) {
for (int k=0; k<dim; k++) f[i][k] -= fcoresum[k];
} else {
if (drudetype[type[i]] == DRUDE_TYPE) continue; // do with the core
int j = atom->map(drudeid[i]);
double mi, mj, mtot; // i is core, j is drude
if (rmass) {
mi = rmass[i];
mj = rmass[j];
} else {
mi = mass[type[i]];
mj = mass[type[j]];
}
mtot = mi + mj;
mi /= mtot;
mj /= mtot;
for (int k=0; k<dim; k++) {
f[i][k] -= mi * fcoresum[k];
f[j][k] -= mj * fcoresum[k];
}
}
}
}
}
// Reverse communication of the forces on ghost Drude particles
comm->reverse_comm();
}
/* ---------------------------------------------------------------------- */
void FixLangevinDrude::reset_target(double t_new)
{
t_target_core = t_start_core = t_new;
}
/* ----------------------------------------------------------------------
extract thermostat properties
------------------------------------------------------------------------- */
void *FixLangevinDrude::extract(const char *str, int &dim)
{
dim = 0;
if (strcmp(str,"t_target_core") == 0) {
return &t_target_core;
} else if (strcmp(str,"t_target_drude") == 0) {
return &t_target_drude;
} else error->all(FLERR, "Illegal extract string in fix langevin/drude");
return NULL;
}
/* ---------------------------------------------------------------------- */
int FixLangevinDrude::pack_reverse_comm(int n, int first, double *buf)
{
int i,m,last;
double ** f = atom->f;
m = 0;
last = first + n;
for (i = first; i < last; i++) {
buf[m++] = f[i][0];
buf[m++] = f[i][1];
buf[m++] = f[i][2];
}
return m;
}
/* ---------------------------------------------------------------------- */
void FixLangevinDrude::unpack_reverse_comm(int n, int *list, double *buf)
{
int i,j,m;
double ** f = atom->f;
m = 0;
for (i = 0; i < n; i++) {
j = list[i];
f[j][0] += buf[m++];
f[j][1] += buf[m++];
f[j][2] += buf[m++];
}
}

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